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 Yverdun as English chaplain, bringing with him some English pupils. At Yverdun he remained nearly three years, mastering Pestalozzi's principles. Returning to England in April 1822, he resolved to devote his life to their introduction into this country. He at once opened a school at Epsom for the purpose of showing their application to the education of the upper classes, and when, in 1826, the number of boys outgrew the accommodation of the house there, he removed to Cheam, where he continued to carry on his school till his death. The undertaking was very successful; boys' names were entered several years before their school age, and on some occasions immediately upon their births. Among his more distinguished pupils may be reckoned Samuel Waldegrave, bishop of Carlisle; Henry Shepheard, fellow of Oriel, and subsequently master of Cheam school; Henry Richards Luard [q. v.], registrary of Cambridge University; and three sons of Sir Thomas Francis Fremantle, first lord Cottesloe. ‘With great earnestness of purpose, in Dr. Mayo's character was combined a sincere and all-absorbing yet somewhat simple piety, which was tinged with the principles of the evangelical revival, while at the same time he was a consistent and loyal son of the Church of England.’ Mayo took every opportunity of expounding Pestalozzi's system, and delivered a lecture on his life at the Royal Institution in May 1826. He also took great interest in the foundation and management of the Home and Colonial Training College in Gray's Inn Road, London, which was intended to show the application of Pestalozzianism to elementary education.

Mayo died 23 Feb. 1846, and was buried at Cheam, where a tablet, erected by pupils and friends, speaks of his work as illustrating, ‘both in theory and practice, the blessings of an education based upon Intellectual Development, Scriptural Teaching, and Christian Influence.’ By his wife Mary, daughter of Edward Walwyn Shepheard, esq., of Great Russell Street, London, he left issue a daughter Mary, and two sons, the Rev. Charles Theodore Mayo, M.A. (1832–1892), vicar of St. Andrew's, Hillingdon, Middlesex, and the Rev. Theodore Mayo, M.A., of Quatford House, Shropshire.

Mayo wrote ‘Observations on the Establishment and Direction of Infant Schools,’ 1827, and ‘Memoirs of Pestalozzi,’ 1828, besides numerous school books and sermons.  MAYO, CHARLES (1767–1858), professor of Anglo-Saxon, born in London 24 March 1767, was second son of, D.D. (1720–1802), by his wife Mary, daughter of George Coldham, surgeon extraordinary to the Prince of Wales. The father (son of Charles Mayo of Hereford) was elected fellow at Brasenose College, Oxford, in 1740 (M.A. 1745, and D.D. 1763), and after serving curacies in the east of London was presented in 1764 to the living of Middleton Cheney, Northamptonshire, which he relinquished the same year to return to the east end of London as rector of St. George's. There he continued till his death. He was J.P. for Middlesex, and treasurer of Raine's Hospital, and was an exemplary parish priest in poor districts at a time not generally noted for spiritual activity.

Charles was admitted to Merchant Taylors' School, 1776, and thence elected to St. John's College, Oxford, 1785, of which society he became fellow in 1788. He graduated M.A. 1793, and B.D. 1796. In 1795 he was elected by the university professor of Anglo-Saxon on the foundation of Dr. Rawlinson, being the first to hold that office, and he occupied it for the allotted space of five years. Dr. Samuel Parr states that his lectures were much applauded. Mayo took holy orders and was Whitehall preacher 1799–1800, and morning lecturer at the old chapel of St. Michael, Highgate, for thirty years. He was elected F.S.A. 1820, F.R.S. 1827, and a governor of Cholmeley School in Highgate 1842. He resided during the greater part of his life at Cheshunt, Hertfordshire, where he inherited in 1824 the manor of Andrewes and Le Motte from his grandmother Rebecca, daughter of Sir John Shaw, bart. He married Louisa, daughter of James Landon, but died without issue 10 Dec. 1858, aged 91 years. He was buried at Cheshunt.

Charles's elder brother, (1766–1836), was elected to a medical fellowship at St. John's College, Oxford, 6 July 1792, and graduated D.M. in 1795. Elected physician to the Middlesex Hospital 23 Aug. 1793, he was admitted F.R.C.P. 30 Sept. 1796, and was censor 1797, Gulstonian lecturer 1798, and Harveian orator 1807. Resigning his hospital appointment in 1801, he removed from Conduit Street, London, to Doncaster, and eventually to Bridlington, where he died 6 July 1836. He married Charlotte, daughter of the Rev. Stephen Buckle, LL.D., and left issue.

[E. Wilson's History of Middlesex Hospital; Munk's Coll. of Phys.; Hist. of Mayo Family, 1882.]  MAYO, CHARLES (1837–1877), army surgeon, born at Winchester 13 Jan. 1837, was elder son of Charles Mayo, F.R.C.S. (1788–